1967 Your Friendly Neighborhood Spider-Man vs The Green Goblin in The Witching Hour

Spider-Man TV Series 1967–1970 TV-Y7 Original cartoon series based on the web-slinging Marvel comic book character, Peter Parker, who, after being bit by a radioactive spider, assumes extraordinary powers.
Creators: Stan Lee, Steve Ditko
Stars: Paul Soles, Peg Dixon, Paul Kligman
S1.E6 The Witching Hour Episode aired Oct 14, 1967 Spider-Man (1967)
The Green Goblin tries to make a pact with J.Jonah Jameson in order to catch Spider-Man. However, Spidey must beware of his foe's witching powers.
Directors: Clyde Geronimi, Sid Marcus, Grant Simmons
Writers: Phil Babet, Al Bertino, Lin Carter
Stars: Bernard Cowan, Paul Kligman, Paul Soles